Effect of surface ligands on gold nanocatalysts for CO2 reduction

Hongyu Shang; Spencer K. Wallentine; Daniel M. Hofmann; Quansong Zhu; Catherine J. Murphy; L. Robert Baker

doi:10.1039/d0sc05089j

journal article Open Access Jan 01, 2020

Effect of surface ligands on gold nanocatalysts for CO2 reduction

Hongyu Shang

Spencer K. Wallentine Daniel M. Hofmann Quansong Zhu

Catherine J. Murphy

L. Robert Baker

Chemical Science Vol. 11 No. 45 pp. 12298-12306 · Royal Society of Chemistry (RSC)

View at Publisher Save 10.1039/d0sc05089j

Abstract

Dodecanethiol on Au nanoparticles significantly enhances selectivity and stability with minimal loss in activity by acting as a CO2-permeable membrane, which blocks the deposition of metal ions that are otherwise responsible for rapid deactivation.

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Metrics

48

Citations

57

References

Details

Published: Jan 01, 2020
Vol/Issue: 11(45)
Pages: 12298-12306
License: View

Authors

H

Hongyu Shang

The Ohio State University, Columbus, Ohio, USA

S

Spencer K. Wallentine

The Ohio State University, Columbus, Ohio, USA

D

Daniel M. Hofmann

University of Illinois at Urbana-Champaign, Urbana, Illinois, USA

Q

Quansong Zhu

The Ohio State University, Columbus, Ohio, USA

C

Catherine J. Murphy

University of Illinois at Urbana-Champaign, Urbana, Illinois, USA

L

L. Robert Baker

The Ohio State University, Columbus, Ohio, USA

Funding

National Science Foundation Award: 1665280

Cite This Article

Hongyu Shang, Spencer K. Wallentine, Daniel M. Hofmann, et al. (2020). Effect of surface ligands on gold nanocatalysts for CO2 reduction. Chemical Science, 11(45), 12298-12306. https://doi.org/10.1039/d0sc05089j

Effect of surface ligands on gold nanocatalysts for CO2 reduction

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