The crucial role of oxygen substitution in argyrodite solid electrolytes from the bulk to the surface under atmospheric conditions

Taesoon Hwang; You-Jin Lee; So Ri Lee; Yoon-Cheol Ha; Maenghyo Cho; Sang-Min Lee; Kyeongjae Cho

doi:10.1039/d2ta03649e

journal article Jan 01, 2022

The crucial role of oxygen substitution in argyrodite solid electrolytes from the bulk to the surface under atmospheric conditions

Taesoon Hwang

You-Jin Lee

So Ri Lee Yoon-Cheol Ha

Maenghyo Cho

Sang-Min Lee

Kyeongjae Cho

Journal of Materials Chemistry A Vol. 10 No. 32 pp. 16908-16919 · Royal Society of Chemistry (RSC)

View at Publisher Save 10.1039/d2ta03649e

Abstract

O substitution for S in argyrodite-type sulfide-based solid electrolytes enhances the stability by suppressing reaction with H2O and decomposition. O substitution modulates the electronic structures and then improves electrochemical performance.

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Citations

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References

Details

Published: Jan 01, 2022
Vol/Issue: 10(32)
Pages: 16908-16919
License: View

Authors

T

Taesoon Hwang

Department of Materials Science and Engineering, University of Texas at Dallas, Richardson 75080, Texas, USA; Department of Mechanical and Aerospace Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea

Y

You-Jin Lee

Battery Research Center, Korea Electrotechnology Research Institute, Seongsan-gu, Changwon-si, 51543, Korea

S

So Ri Lee

Battery Research Center, Korea Electrotechnology Research Institute, Seongsan-gu, Changwon-si, 51543, Korea

Y

Yoon-Cheol Ha

Battery Research Center, Korea Electrotechnology Research Institute, Seongsan-gu, Changwon-si, 51543, Korea

M

Maenghyo Cho

Department of Mechanical and Aerospace Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea

S

Sang-Min Lee

Battery Research Center, Korea Electrotechnology Research Institute, Seongsan-gu, Changwon-si, 51543, Korea; Graduate Institute of Ferrous & Energy Materials Technology, Pohang University of Science and Technology, 77 Cheongam-Ro, Nam-Gu, Pohang-si 37673, Republic of Korea

K

Kyeongjae Cho

Department of Materials Science and Engineering, University of Texas at Dallas, Richardson 75080, Texas, USA

Funding

Ministry of Trade, Industry and Energy

Korea Electrotechnology Research Institute Award: 22A01011

Cite This Article

Taesoon Hwang, You-Jin Lee, So Ri Lee, et al. (2022). The crucial role of oxygen substitution in argyrodite solid electrolytes from the bulk to the surface under atmospheric conditions. Journal of Materials Chemistry A, 10(32), 16908-16919. https://doi.org/10.1039/d2ta03649e

The crucial role of oxygen substitution in argyrodite solid electrolytes from the bulk to the surface under atmospheric conditions

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