19.46%-Efficiency all-polymer organic solar cells with excellent outdoor operating stability enabled by active layer reconstruction

Layer-by-layer blade deposition was employed along with a multi-component strategy to construct a quaternary all-polymer system, achieving a high power conversion efficiency of 19.46% and improved outdoor operating stability.

Topics

No keywords indexed for this article. Browse by subject →

References

69

[1]

Z. G.Zhang and Y.Li , Angew. Chem., Int. Ed. , 2021 , 60 , 4422–4433

[2]

Wang Chin. J. Polym. Sci. (2022) 10.1007/s10118-022-2697-1

[3]

Shao Adv. Mater. (2023) 10.1002/adma.202208750

[4]

Zhan Adv. Mater. (2022) 10.1002/adma.202206269

[5]

Zhu Nat. Mater. (2022) 10.1038/s41563-022-01244-y

[6]

Zheng Joule (2022) 10.1016/j.joule.2021.12.017

[7]

Z. G.Zhang , Y.Yang , J.Yao , L.Xue , S.Chen , X.Li , W.Morrison , C.Yang and Y.Li , Angew. Chem., Int. Ed. , 2017 , 56 , 13503–13507

[8]

Gao Sci. China: Chem. (2023) 10.1007/s11426-023-1720-x

[9]

Yang Adv. Mater. (2022) 10.1002/adma.202209350

[10]

Sun Joule (2021) 10.1016/j.joule.2021.04.007

[11]

Yu Adv. Mater. (2022) 10.1002/adma.202200361

[12]

Wu Natl. Sci. Rev. (2022) 10.1093/nsr/nwab151

[13]

Dong Joule (2020) 10.1016/j.joule.2020.07.028

[14]

Sun Joule (2020) 10.1016/j.joule.2019.12.004

[15]

Morphology Control in Organic Solar Cells

Fuwen Zhao, Chunru Wang, Xiaowei Zhan

Advanced Energy Materials 2018 10.1002/aenm.201703147

[16]

Gao Adv. Mater. (2016) 10.1002/adma.201504629

[17]

Song Matter (2022) 10.1016/j.matt.2022.08.011

[18]

Song Adv. Mater. (2024) 10.1002/adma.202406922

[19]

Li J. Am. Chem. Soc. (2016) 10.1021/jacs.6b04822

[20]

Zhu Adv. Mater. (2019) 10.1002/adma.201902899

[21]

Fu Adv. Mater. (2022) 10.1002/adma.202202608

[22]

Sun Energy Environ. Sci. (2019) 10.1039/c8ee02560f

[23]

Sun Energy Environ. Sci. (2019) 10.1039/c9ee02295c

[24]

Sun Joule (2022) 10.1016/j.joule.2022.10.005

[25]

Xu Adv. Mater. (2023) 10.1002/adma.202208997

[26]

Wang Nat. Energy (2024) 10.1038/s41560-023-01436-z

[27]

Zhu Joule (2024) 10.1016/j.joule.2024.08.001

[28]

Sun Nat. Energy (2022) 10.1038/s41560-022-01140-4

[29]

Wu Adv. Funct. Mater. (2021) 10.1002/adfm.202010411

[30]

Sun Joule (2023) 10.1016/j.joule.2022.12.007

[31]

Ma Energy Environ. Sci. (2025) 10.1039/d4ee02978j

[32]

Zeng Nat. Commun. (2023) 10.1038/s41467-023-39832-4

[33]

Wang J. Energy Chem. (2024) 10.1016/j.jechem.2024.05.010

[34]

Fan Sci. China: Chem. (2018) 10.1007/s11426-017-9199-1

[35]

Qin J. Semicond. (2021) 10.1088/1674-4926/42/1/010501

[36]

Fu Sci. China: Chem. (2021) 10.1007/s11426-021-1140-x

[37]

Jia Nano Energy (2020) 10.1016/j.nanoen.2020.104718

[38]

Fan Energy Environ. Sci. (2020) 10.1039/d0ee01828g

[39]

Wang Joule (2020) 10.1016/j.joule.2020.03.019

[40]

Ma Adv. Mater. (2023) 10.1002/adma.202208926

[41]

Sun Sol. RRL (2020) 10.1002/solr.202000156

[42]

Hsieh ACS Appl. Mater. Interfaces (2017) 10.1021/acsami.7b01296

[43]

Simultaneous enhanced efficiency and thermal stability in organic solar cells from a polymer acceptor additive

Wenyan Yang, Zhenghui Luo, Rui Sun et al.

Nature Communications 2020 10.1038/s41467-020-14926-5

[44]

Liu Angew. Chem., Int. Ed. (2023) 10.1002/anie.202316039

[45]

Dou Adv. Energy Mater. (2024) 10.1002/aenm.202402268

[46]

Luke Nat. Rev. Mater. (2023) 10.1038/s41578-023-00606-5

[47]

Ghasemi Nat. Mater. (2021) 10.1038/s41563-020-00872-6

[48]

F.Yi , M.Xiao , Y.Meng , H.Bai , W.Su , W.Gao , Z. F.Yao , G.Qi , Z.Liang , C.Jin , L.Tang , R.Zhang , L.Yan , Y.Liu , W.Zhu , W.Ma and Q.Fan , Angew. Chem., Int. Ed. , 2024 , 63 , 202319295

[49]

Zhang Joule (2024) 10.1016/j.joule.2023.12.009

[50]

Dou Joule (2024) 10.1016/j.joule.2024.10.006

Showing 50 of 69 references

Cited By

49

Small-Molecule Donor/Polymer Acceptor-Based Organic Solar Cells Achieve >10% Efficiency

Dashun Huang, Zhihao Chen · 2025

ACS Applied Materials & Interfa...

Metrics

49

Citations

69

References

Details

Published: Jan 01, 2025
Vol/Issue: 18(4)
Pages: 1812-1823
License: View

Authors

X

Xiaohei Wu

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China

B

Bo Xiao

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China

R

Rui Sun

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China; Institute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, China; Key Laboratory of Advanced Electrode Materials for Novel Solar Cells for Petroleum and Chemical Industry of China, School of Chemistry and Life Sciences, Suzhou University of Science and Technology, Suzhou 215009, China

X

Xinrong Yang

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China

M

Meimei Zhang

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China

Y

Yuan Gao

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China

B

Biao Xiao

Key Laboratory of Optoelectronic Chemical Materials and Devices (Ministry of Education), School of Optoelectronic Materials & Technology, Jianghan University, Wuhan 430056, China

E

Elizaveta D. Papkovskaya

Enikolopov Institute of Synthetic Polymeric Materials of the Russian Academy of Sciences, Moscow 117393, Russia

Y

Yuriy Luponosov

Enikolopov Institute of Synthetic Polymeric Materials of the Russian Academy of Sciences, Moscow 117393, Russia

C

Christoph J. Brabec

Institute of Materials for Electronics and Energy Technology (i-MEET), Department of Materials Science and Engineering, Friedrich-Alexander-Universität Erlangen-Nürnberg, Erlangen 91058, Germany

J

Jie Min

The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China

Funding

National Natural Science Foundation of China Award: 22279094

Fundamental Research Funds for the Central Universities

Natural Science Foundation of Hubei Province Award: 2024AFB068

South China University of Technology Award: 2024-skllmd-23

Cite This Article

Xiaohei Wu, Bo Xiao, Rui Sun, et al. (2025). 19.46%-Efficiency all-polymer organic solar cells with excellent outdoor operating stability enabled by active layer reconstruction. Energy Environ. Sci., 18(4), 1812-1823. https://doi.org/10.1039/d4ee05083e

19.46%-Efficiency all-polymer organic solar cells with excellent outdoor operating stability enabled by active layer reconstruction

You May Also Like