Research Progress on Coating Structure of Silicon Anode Materials for Lithium‐Ion Batteries

Ke Xu; Xuefeng Liu; Keke Guan; Wen Lei; Shaowei Zhang; Quanli Jia; Haijun Zhang

doi:10.1002/cssc.202101837

journal article Oct 25, 2021

Research Progress on Coating Structure of Silicon Anode Materials for Lithium‐Ion Batteries

Ke Xu

Xuefeng Liu

Keke Guan Wen Lei

Shaowei Zhang Quanli Jia Haijun Zhang

ChemSusChem Vol. 14 No. 23 pp. 5135-5160 · Wiley

View at Publisher Save 10.1002/cssc.202101837

Abstract

AbstractSilicon, which has been widely studied by virtue of its extremely high theoretical capacity and abundance, is recognized as one of the most promising anode materials for the next generation of lithium‐ion batteries. However, silicon undergoes tremendous volume change during cycling, which leads to the destruction of the electrode structure and irreversible capacity loss, so the promotion of silicon materials in commercial applications is greatly hampered. In recent years, many strategies have been proposed to address these shortcomings of silicon. This Review focused on different coatings materials (e. g., carbon‐based materials, metals, oxides, conducting polymers, etc.) for silicon materials. The role of different types of materials in the modification of silicon‐based material encapsulation structure was reviewed to confirm the feasibility of the protective layer strategy. Finally, the future research direction of the silicon‐based material coating structure design for the next‐generation lithium‐ion battery was summarized.

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Details

Published: Oct 25, 2021
Vol/Issue: 14(23)
Pages: 5135-5160
License: View

Authors

K

Ke Xu

The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and Technology Wuhan 430081 P. R. China

X

Xuefeng Liu

The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and Technology Wuhan 430081 P. R. China

K

Keke Guan

The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and Technology Wuhan 430081 P. R. China

W

Wen Lei

The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and Technology Wuhan 430081 P. R. China

S

Shaowei Zhang

College of Engineering, Mathematics and Physical Sciences University of Exeter Exeter EX4 4QF United Kingdom

Q

Quanli Jia

Henan Key Laboratory of High Temperature Functional Ceramics Zhengzhou University Zhengzhou 450052 Henan P. R. China

H

Haijun Zhang

The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and Technology Wuhan 430081 P. R. China

Funding

National Natural Science Foundation of China Award: 51872210

Cite This Article

Ke Xu, Xuefeng Liu, Keke Guan, et al. (2021). Research Progress on Coating Structure of Silicon Anode Materials for Lithium‐Ion Batteries. ChemSusChem, 14(23), 5135-5160. https://doi.org/10.1002/cssc.202101837

Research Progress on Coating Structure of Silicon Anode Materials for Lithium‐Ion Batteries

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